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Security was tightened at Jewish sites across Belgium following the killings.
Brussels Jewish Museum shooting – The suspect
Belgian police earlier released security camera footage showing the suspect they were hunting
He was arrested during a customs check at the Saint-Charles train station in the southern French city of Marseille on Friday.
He had been on board a bus that was travelling from Amsterdam via Brussels, AFP news agency reports.
Belgium has a Jewish population of some 42,000, about half of whom live in the capital